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Nd-Fe-B磨削油泥 1

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厌氧消化，生物固体，污染，甲基苯丙胺，吸附 1

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污水厂污泥；污泥处理；污染控制；资源回收；减污降碳 1

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Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 886-896 doi: 10.1007/s11705-021-2125-z

摘要： Supercritical water gasification is a promising technology in dealing with the degradation of hazardous waste, such as oily sludge, accompanied by the production of fuel gases. To evaluate the mechanism of Fe2O3 catalyst and the migration pathways of heteroatoms and to investigate the systems during the process, reactive force field molecular dynamics simulations are adopted. In terms of the catalytic mechanisms of Fe2O3, the surface lattice oxygen is consumed by small carbon fragments to produce CO and CO2, improving the catalytic performance of the cluster due to more unsaturated coordination Fe sites exposed. Lattice oxygen combines with •H radicals to form water molecules, improving the catalytic performance. Furthermore, the pathway of asphaltene degradation was revealed at an atomic level, as well as products. Moreover, the adsorption of hydroxyl radical on the S atom caused breakage of the two C–S bonds in turn, forming •HSO intermediate, so that the organic S element was fixed into the inorganic liquid phase. The heteroatom O was removed under the effects of supercritical water. Heavy metal particles presented in the oily sludge, such as iron in association with Fe2O3 catalyst, helped accelerate the degradation of asphaltenes.

关键词： oily sludge     SCWG     ReaxFF     Fe2O3     heteroatoms    

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Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1570-3

摘要：

● Collaborative treatment of plastics and OS was established to improve oil quality.

关键词： Oily sludge     Pyrolysis     Polyethylene     H/Ceff ratio     Oil quality    

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Comparison of CNT-PVA membrane and commercial polymeric membranes in treatment of emulsified oily wastewater

Gang Yi, Xinfei Fan, Xie Quan, Shuo Chen, Hongtao Yu

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1103-x

摘要：

CNT-PVA membrane was fabricated and compared with polymeric membranes.

The separation performance was evaluated by homemade and cutting fluid emulsions.

The three membranes show similar oil retention rates.

CNT-PVA membranes have higher permeation fluxes compared with polymeric membranes.

CNT-PVA membrane shows higher fouling resistance.

关键词： Oily wastewater     Microfiltration     Carbon nanotube membrane     Commercial polymeric membrane    

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Bioinspired cellulose-based membranes in oily wastewater treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1515-2

摘要：

• Cellulose-based membrane separates oily wastewater mimicking the living things.

关键词： Cellulose     Bioinspired membrane     Superhydrophobic surface     Underwater superoleophobic surface     Oil-water separation    

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Comparison between inhibitor and uncoupler for minimizing excess sludge production of an activated sludge

CHEN Guowei, XI Pengge, XU Deqian, YU Hanqing

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 63-66 doi: 10.1007/s11783-007-0012-6

摘要： In order to study the minimization of excess sludge production, the reduction in the excess sludge production in the presence of an inhibitor and uncoupler was studied in this work. The experimental results show that such an addition could effectively reduce the production of excess sludge. With the energy uncoupling model established in this work, energy uncoupling coefficient () was used to evaluate the reduction in excess sludge production. The energy uncoupling coefficients in the presence of dinitrophenol (dNP), Zn, and Cu was 0.75, 0.46, and 0.18, respectively. The analysis demonstrated that energy spilling occurred in the presence of dNP, and that dNP was an effective uncoupler for reducing the production of excess activated sludge without affecting the microbial respiration activity.

关键词： uncoupling coefficient     Cu     minimization     presence     uncoupling    

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Preparation and characterization of hydrothermally engineered TiO

Kanchapogu Suresh, G. Pugazhenthi, R. Uppaluri

《化学科学与工程前沿（英文）》 2017年 第11卷 第2期   页码 266-279 doi: 10.1007/s11705-017-1608-4

摘要： This work targets the preparation and characterization of an inexpensive TiO -fly ash composite membrane for oily wastewater treatment. The composite membrane was fabricated by depositing a hydrophilic TiO layer on a fly ash membrane via the hydrothermal method, and its structural, morphological and mechanical properties were evaluated. The separation potential of the composite membrane was evaluated for 100–200 mg·L synthetic oily wastewater solutions. The results show that the composite membrane has excellent separation performance and can provide permeate stream with oil concentration of only 0.26–5.83 mg·L . Compared with the fly ash membrane in the average permeate flux and performance index (49.97 × 10 m ·m ·s and 0.4620%, respectively), the composite membrane exhibits better performance (51.63 × 10 m ·m ·s and 0.4974%). For the composite ash membrane, the response surface methodology based analysis inferred that the optimum process parameters to achieve maximum membrane flux and rejection are 207 kPa, 200 mg·L and 0.1769 m·s for applied pressure, feed concentration and cross flow velocity, respectively. Under these conditions, predicted responses are 41.33 × 10 m ·m ·s permeate flux and 98.7% rejection, which are in good agreement with the values obtained from experimental investigations (42.84 × 10 m ·m ·s and 98.82%). Therefore, we have demonstrated that the TiO -fly ash composite membrane as value added product is an efficient way to recycle fly ash and thus mitigate environmental hazards associated with the disposal of oily wastewaters.

关键词： TiO2-fly ash membrane     oily wastewater     fouling     microfiltration    

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Co-pyrolysis of sludge and kaolin/zeolite in a rotary kiln: Analysis of stabilizing heavy metals

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1488-1

摘要：

• Adding kaolin/zeolite promotes the formation of stable heavy metals.

关键词： Co-pyrolysis     Sewage sludge     Heavy metals     Rotary kiln     Immobilization mechanism    

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Cultivation of aerobic granular sludge in a conventional, continuous flow, completely mixed activatedsludge system

Xi CHEN,Linjiang YUAN,Wenjuan LU,Yuyou LI,Pei LIU,Kun NIE

《环境科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 324-333 doi: 10.1007/s11783-014-0627-3

摘要： Aerobic granules were formed in a conventional, continuous flow, completely mixed activated sludge system (CMAS). The reactor was inoculated with seed sludge containing few filaments and fed with synthetic municipal wastewater. The settling time of the sludge and the average dissolved oxygen (DO) of the reactor were 2 h and 4.2 mg·L , respectively. The reactor was agitated by a stirrer, with a speed of 250 r·min , to ensure good mixing．The granular sludge had good settleability, and the sludge volume index (SVI) was between 50 and 90 mL·g . The laser particle analyzer showed the diameter of the granules to be between 0.18 and 1.25 mm. A scanning electron microscope (SEM) investigation revealed the predominance of sphere-like and rod-like bacteria, and only few filaments grew in the granules. The microbial community structure of the granules was also analyzed by polymerase chain reaction-denaturing gradient gel electrophoresis (PCR-DGGE). Sequencing analysis indicated the dominant species were α, β, and γ- , , and . The data from the study suggested that aerobic granules could form, if provided with sufficient number of filaments and high shear force. It was also observed that a high height-to-diameter ratio of the reactor and short settling time were not essential for the formation of aerobic granular sludge.

关键词： aerobic granular sludge     completely mixed activated sludge system (CMAS)     continuous flow     shear force     filamentous bacteria     polymerase chain reaction-denaturing gradient gel electrophoresis (PCR-DGGE)    

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Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第6期   页码 884-891 doi: 10.1007/s11783-012-0408-9

摘要： Low dissolved oxygen (DO) is an energy-saving condition in activated sludge process. To investigate the possible application of limited filamentous bulking (LFB) in sequencing batch reactor (SBR), two lab-scale SBRs were used to treat synthetic domestic wastewater and real municipal wastewater, respectively. The results showed that prolonging low DO aeration duration and setting pre-anoxic (anaerobic) phase were effective strategies to induce and inhibit filamentous sludge bulking, respectively. According to the sludge settleability, LFB could be maintained steadily by adjusting operation patterns. Filamentous bacteria content and sludge volume index (SVI) were likely correlated. SVI fluctuated dramatically within a few cycles when around 200 mL·g , where altering operation pattern could change sludge settleability in spite of the unstable status of activated sludge system. Energy consumption by aeration reduced under low DO LFB condition, whereas the nitrification performance deteriorated. However, short-cut nitrification and simultaneous nitrification denitrification (SND) were prone to take place under such conditions. When the cycle time kept constant, the anoxic (anaerobic) to aerobic time ratio was determining factor to the SND efficiency. Similarity keeping aerobic time as constant, the variation trends of SND efficiency and specific SND rate were uniform. SBR is a promising reactor to apply the LFB process in practice.

关键词： limited filamentous bulking     sequencing batch reactor     sludge settleability     sludge volume index     simultaneous nitrification denitrification    

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High-solid anaerobic digestion of sewage sludge: achievements and perspectives

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1364-4

摘要：

• High-solid anaerobic digestion (HS-AD) of sewage sludge (SS) is overviewed.

关键词： High-solid effect     Anaerobic fermentation     Methane production     Biodegradability     Sludge treatment    

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A review on sustainable reuse applications of Fenton sludge during wastewater treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1511-6

摘要：

• The sustainable approaches related to Fenton sludge reuse systems are summarized.

关键词： Fenton sludge     Heavy metals     Coagulant     Iron source     Heterogeneous catalyst    

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Properties and effect of forming sewage sludge into lightweight ceramics

Min YUE, Qinyan YUE, Yuanfeng QI, Baoyu GAO, Hui YU

《环境科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 117-124 doi: 10.1007/s11783-010-0220-3

摘要： In this work we investigated the chemical, thermal and toxic properties of dried sewage sludge (DSS), the preparation and properties of lightweight sludge ceramic (LSC) and the mechanisms of action of the organic and inorganic foaming agents (OFAs and IFAs). The chemical components and thermal properties of the raw materials were studied by Energy Dispersive X-ray Detection (EDX) and Thermogravimetric Analysis and Differential Scanning Calorimetry (DSC/TGA). The mineral phases of the raw materials and the formed ceramics were determined by X-ray Diffraction (XRD). The leaching characteristics of heavy metals were investigated with Inductively Coupled Plasma Atomic Emission Spectrometry (ICP-AES). Different ratios of DSS and clay were mixed and pressed into raw pellets. After drying and preheating treatment, the raw pellets were sintered at 1150°C for 10 min. The physical properties of LSC (50 wt% DSS added) were tested. The results showed that when the addition of DSS was above 50 wt%, LSC began to shrink, and a maximum density occurred. The environmental safety of LSC was satisfactory. XRD showed that some new mineral phases formed in the LSC. Observation of the microstructure by Scanning Electron Microscope (SEM) indicated that the body of LSC was porous.

关键词： sludge     foaming agents     ceramics     preheating process    

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Effect of wastewater composition on the calcium carbonate precipitation in upflow anaerobic sludge blanket

Shucheng YANG, Yanling HE, Charles CHOU, Pengxiang ZHANG, Dongqi WANG, Yonghong LIU,

《环境科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 142-149 doi: 10.1007/s11783-010-0026-3

摘要： Calcium carbonate often precipitates in anaerobic reactors treating wastewater with high calcium content. The aim of this paper is to study the effect of wastewater composition on calcium carbonate precipitation in upflow anaerobic sludge blanket (UASB) reactors. Two laboratory-scale UASB reactors were operated with calcium-containing influents using acetate and carbohydrate as substrate, respectively. There was an obvious accumulation of inorganic precipitate observed in the biogranules. Observations via scanning electron microscope (SEM) and energy dispersive spectroscopy (EDS) showed that the acclimated biogranules in the two reactors differed in microstructure. Calcium carbonate was found to have precipitated on the surface of acetate-degrading biogranules, but precipitated at the core of the carbohydrate-degrading biogranules. The results indicated that substrates had significant influence on the location of calcium carbonate precipitation in anaerobic granular sludge, which was expected due to the different methanogens distribution and pH gradient within the granular sludge degrading various substrates. Moreover, the location of calcium carbonate precipitation substantially affected the specific methanogenic activity (SMA) of the granular sludge. The SMA of the acetate-degrading biogranules dropped from 1.96 gCOD·gVSS·d to 0.61 gCOD·gVSS·d after 180-d of operation in the reactor. However, the SMA of the carbohydrate-degrading biogranules was not adversely affected by calcium carbonate precipitation.

关键词： calcium carbonate     precipitation     anaerobic granular sludge     wastewater composition     microstructure     upflow anaerobic sludge blanket (UASB)    

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New insights into different surfactants’ impacts on sludge fermentation: Focusing on the particular metabolic

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1527-6

摘要：

• The promoting effects for VFA generation follow the order of APG>SDBS>HTAB.

关键词： Waste activated sludge (WAS)     Volatile fatty acids (VFA)     Surfactant types     Functional microorganisms     Metabolic activity upregulation    

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Fate of proteins of waste activated sludge during thermal alkali pretreatment in terms of sludge protein

Xiaoli Song, Zhenghua Shi, Xiufen Li, Xinhua Wang, Yueping Ren

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1114-7

摘要：

Maillard reaction between reducing sugars and amides happened during pretreatment.

Over 90 min of TAH at the optimal condition, 67.59% sludge proteins was solubilized.

15.84% soluble proteins broke down to materials with small molecular weight.

关键词： Sludge flocs     Microbial cells     Hydrolysate     Protein breakdown     Melanoidin    

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标题 作者 时间 类型 操作

Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

期刊论文

Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis

期刊论文

Comparison of CNT-PVA membrane and commercial polymeric membranes in treatment of emulsified oily wastewater

Gang Yi, Xinfei Fan, Xie Quan, Shuo Chen, Hongtao Yu

期刊论文

Bioinspired cellulose-based membranes in oily wastewater treatment

期刊论文

Comparison between inhibitor and uncoupler for minimizing excess sludge production of an activated sludge

CHEN Guowei, XI Pengge, XU Deqian, YU Hanqing

期刊论文

Preparation and characterization of hydrothermally engineered TiO

Kanchapogu Suresh, G. Pugazhenthi, R. Uppaluri

期刊论文

Co-pyrolysis of sludge and kaolin/zeolite in a rotary kiln: Analysis of stabilizing heavy metals

期刊论文

Cultivation of aerobic granular sludge in a conventional, continuous flow, completely mixed activatedsludge system

Xi CHEN,Linjiang YUAN,Wenjuan LU,Yuyou LI,Pei LIU,Kun NIE

期刊论文

Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

期刊论文

High-solid anaerobic digestion of sewage sludge: achievements and perspectives

期刊论文

A review on sustainable reuse applications of Fenton sludge during wastewater treatment

期刊论文

Properties and effect of forming sewage sludge into lightweight ceramics

Min YUE, Qinyan YUE, Yuanfeng QI, Baoyu GAO, Hui YU

期刊论文

Effect of wastewater composition on the calcium carbonate precipitation in upflow anaerobic sludge blanket

Shucheng YANG, Yanling HE, Charles CHOU, Pengxiang ZHANG, Dongqi WANG, Yonghong LIU,

期刊论文

New insights into different surfactants’ impacts on sludge fermentation: Focusing on the particular metabolic

期刊论文

Fate of proteins of waste activated sludge during thermal alkali pretreatment in terms of sludge protein

Xiaoli Song, Zhenghua Shi, Xiufen Li, Xinhua Wang, Yueping Ren

期刊论文